No - DataTables requires data to be given to it in a known format. The reason for this is that everyone would have a different format (e.g. I had no idea what you would give it an array with a key called 'ResultSet', and sub fields called 'Field1' etc!) - so there needs to be a standard that DataTables understands. This standard is simply a 2D data array (the key being aaData). You can use Javascript to transform from your ResultSet to the DataTables standard if you want.
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Regards,
Allan